Easy Access to Modified Cyclodextrins by an Intramolecular Radical Approach

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Easy access to modified cyclodextrins by an intramolecular radical approach.

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Easy Access to Modified Cyclodextrins via an Intramolecular Radical Approach

A simple methodology to modify the primary face of cyclodextrins (CDs) is described. The 6-O-yl radical of α-, β-, and γCD abstracts regioselectively the H5, located in the adjacent Dglucose unit, by an intramolecular 1,8-hydrogen atom transfer reaction through a geometrically restricted nine-membered transition state to give a stable 1,3,5-trioxocane ring. The reaction has been extended to 1,4...

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ژورنال

عنوان ژورنال: Angewandte Chemie

سال: 2015

ISSN: 0044-8249

DOI: 10.1002/ange.201412300